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Are you speaking of Artifacts which open the vault (plot items) or Artifacts which you can use to improve your action skill?

Those which open the vault can be found in silver chests along plot missions, one is found at Sledge's Safehouse, another at Krom's Canyon, I can't remember where the last is, but if you continue with plot missions you'll find it (open chests after you kill bosses).

Artifacts which improve your action skill can be found in many places, here are some places where they drop:

Note: 1st PT - First Playthrough | 2nd PT - Second Playthrough

Quest Rewards

   * Level 1 Shock : 1st Playthrough Quest Reward for "Shock Crystal Harvest" 
   * Level 1 Fire: 1st Playthrough Quest Reward for "The Legend Of Moe and Marley" 
   * Level 1 Corrosive: 1st Playthrough Quest Reward for "Corrosive Crystal Harvest" 
   * Level 2 Explosive : 1st Playthrough Quest Reward for "Ghost of the Vault" 
   * Level 3 Explosive: 1st Playthrough Quest Reward for "Another Piece Of The Puzzle"
   * Level 4 Fire: 2nd Playthrough Quest Reward for "The Legend Of Moe and Marley" 
   * Level 4 Shock : 2nd Playthrough Quest Reward for "Shock Crystal Harvest" 
   * Level 4 Explosive : 2nd Playthrough Quest Reward for "Ghosts of the Vault" 
   * Level 4 Corrosive: 2nd Playthrough Quest reward for "Corrosive Crystal Harvest" **
   * Level 5 Fire: 2nd Playthrough Quest Reward for "Another Piece Of The Puzzle" 

Drops and Chests

   * Level 1 Explosive: Dropped by Marley while completing "The Legend Of Moe and Marley" during 1st PT.
   * Level 6 Corrosive: Loot-able from SuperBad Poison Scythid after 2nd PT.
   * Level 6 All types: Loot-able from the three wolf mini bosses in the Dr. Ned's Zombie Island DLC after 2nd PT
   * Level 6 All types: Loot-able from The Destroyer, or Scar in Skag Gully after 2nd PT.

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